Physicists headed up by a team at the University of Tennessee, Knoxville, and the Radioactive Isotope Beam Factory (RIBF) at RIKEN in Japan say they have measured the alpha decay of tellurium-104 for the first time. The feat could help us better understand how alpha particles form inside atomic nuclei, which is one of the least understood problems in nuclear science.
Alpha radioactivity was discovered over 125 years ago and it is the process whereby an atomic nucleus emits an alpha particle, which is a helium nucleus consisting of two protons and two neutrons that are strongly bound. The alpha particle exits the nucleus by quantum-mechanical tunnelling through the energy barrier surrounding the nucleus. While this model broadly explains the lifetimes of radioactive nuclei, a big question remains, however, says study lead Robert Grzywacz at the University of Tennessee, Knoxville. This is: how do alpha particles form in the nucleus and where can they exist as “pre-formed” structures inside it before they leave?
Tellurium-104 is particularly suited to studying alpha radioactivity, he says, because it is predicted to have the highest chance of pre-forming alpha particles of all heavy nuclei. “Such a strong enhancement of preformation shouldn’t be possible in theory because the matter in heavy nuclei is uniformly distributed,” Grzywacz explains. “There must, therefore, be an extra mechanism that causes alpha particles to locally ‘clump’ or ‘cluster’.”
In their experiments, he and his colleagues set about measuring the alpha particles produced by tellurium-104. This was no easy task because this isotope of tellurium can only be observed during the decay of xenon-108, which itself is extremely difficult to make in the laboratory.
Pulses of alpha particles
The researchers did their work at Japan’s RIKEN accelerator complex, which consists of four coupled cyclotrons that accelerate a beam of xenon-124 onto a beryllium production target. The collisions between the two produces xenon-108 and then tellurium-104. The tellurium-104 finally decays into tin-100.
Grzywacz and co-workers say they succeeded measuring pulses of alpha particles produced in short succession by the tellurium-104. They measured the half-life of the radioisotope as being 7.2 ns, which is the shortest known alpha decay half-life for alpha particle emission from a heavy nucleus. More importantly, when corrected for the tunnelling effect – using a parameter known as the reduced width, which separates quantum tunnelling from inherent alpha particle emission from the nucleus – they were able to confirm that the probability of an alpha particle pre-forming in the nucleus was much higher than expected from theory calculations.
The possibility that tellurium-104 could show such “superallowed” alpha decay was first put forward more than 60 years ago, but it has been impossible to observe experimentally, says Grzywacz. “We started our search for this decay more than 20 years ago at Oak Ridge National Laboratory and later at JAEA in Tokai (Japan). We proposed the present experiment in 2018 at RIKEN but because of the covid-19 pandemic, we had to repeat the proposal in 2022. The experiment was deemed to be of ‘very high priority’ and we performed our experiments almost exactly two years ago, in June 2024.”
Alpha clusters found on neutron-rich surfaces of nuclei
The work, which is detailed in Nature, will be important for understanding how alpha particle form in nuclei and will push the theory to explain where and how nuclear cluster can form, says Grzywacz. “More than 300 nuclei – and importantly, almost all superheavy nuclei – decay via alpha particle emission. Lighter nuclei may also naturally form ‘alpha condensates’, but in heavier nuclei, it is not obvious how this happens.”
Grzywacz told Physics World that he and his colleagues will now need to measure alpha particle energies with better precision in order to constrain the preformation they have observed.
